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Extra info for The Atmosphere and Ionosphere: Elementary Processes, Discharges and Plasmoids
5 Chemo-Ionization Involving Atoms in Low-Lying Excited States Let us now discuss the experimental facts accumulated over the past two decades that are an illustration of the theory just presented and put it ahead of fundamentally new problems. Therefore it is natural that we begin with a presentation of the results obtained for the AI and PI reactions involving atoms in low-lying excited states. 1 Pair Collisions of Metastable Atoms of Inert Gases Shock radiation kinetics of plasma taking into account the electron–atom and photo processes does not overlap all possible types of the charged particle balance in the plasma.
2B is of the order of the oscillation frequency ! (B is the rotational constant of the molecular ion), where there is no reason to exclude the vibrational degrees of freedom from general consideration. Moreover, most highly excited Rydberg molecular states considered by Lombardi and Seligman (1993) are the autoionization states (see Fig. 6). The dynamics of electron behavior for these states is described in terms of the scattering theory, where the energy eigenvalues and corresponding wave functions are complex (Golubkov and Ivanov 2001).
Let us consider the main types of the symmetrical collisions for this case, which include (1) the chemoionization process in pair collisions of the excited atoms, ( A CA ! N. Bezuglov et al. Fig. 1:61/ ˆ < A2 C e ; C A CA! 1:63/ A CA : At the same time there is a wide range of conditions in which the collisional processes involving atoms in the emitting states can give a significant contribution to the ionization. Thus, an ensemble of the excited states formed in an absorbing medium, irradiated by light, in general, is a potential source of the processes leading to the ionization.